Alright, so I finally got around to having my ECU tuned by the folks at GDE.
First impressions: Like everyone else, WOW! There is a lot more power under the hood now. Once I adjust my driving style for this new found torque/hp, I might stop roaring up hills around town

.
I ran my CRD about 40 miles on the highway, just to get a feel for how she drives now. Conditions were nasty - wind and rain, the whole way. Nevertheless, EVIC showed 37.2mpg when I got off and was still climbing about .1 mpg every mile or so. I know it isn't an accurate read, but that number is fully 6 mpg higher than what the EVIC read on my best tank pre-GDE (that tank hand calculated to 27.8., my EVIC is terrible....)
Now for the fun part. I plan to drive from FL to AZ in a little over two weeks, that's about 2,000 miles. Between now and then, I will be doing a number of things to optimize my Jeep's fuel economy. As I go along, I will update this with what I have done.
Pre-8/1: Bone stock 2006 Limited KJ CRD. Does have the full Mopar skids, which may help mpg slightly.
8/1: GDE Tune, unplugged fuel heater, Amsoil EA 201 Filter, Filterminder
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EDIT 8/4:
Removed and cleaned the MAP today. It was so encrusted that I couldn't even see the frame around the sensor. That couldn't be good

. It's nice and shiny now though!
I also disconnected both CAC(intercooler) hoses and cleaned them out thoroughly. The one running from the intercooler back into the engine block was pretty much clean. The one running from the MAP to the intercooler though? YIKES! It was entirely covered in black sooty oil. Both are now almost good as new. Fortunately they weren't too soggy, so no need to replace them at the moment.
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EDIT 8/7
My Magnaflow #12226 showed up today. I got it from magnaflowperformanceexhausts dot com for just $58 with free shipping. They were a little slow, but you can't beat the price. I've also found a shop that will do the hack/weld job for $35-40. I like mods that come in under $100

.
Looks like I'm averaging about 28mpg in town so far. Where I currently am (not Tempe) is hilly as all get out and 35 mph everywhere. Combined with my short commute (5-6 miles), 28 wouldn't be half bad!
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Edit 8/13
Got the Magnaflow installed today for just $40, not a bad deal. Even with the GDE tune, there is a noticeable difference in drivability. I can climb hills, maintaining speed, at about 100 less RPMs than before, which should translate to better mileage.
GDE + removing engine break = GOBS of coasting ability

I've got so much now that I can coast around 1100RPMs at 35mph and not slow down! It's fantastic!
This concludes my pre-trip mods (with the exception of a radio fix on Saturday

).
Remaining in consideration:
1) Running B25-30 once I get back home, with a fuel filter change after 2-3 tanks. I will do this and the cleaner engine should improve performance slightly
2) Lift pump? Not sure yet, debating with myself....
3) CCV filter of some sort, dependent upon how gross my hoses and MAP sensor are at the next 2 oil changes.
I should have some numbers next week!
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Edit 8/14
First tank mileage: 25.4 hand calculated & adjusted for odo error.
Not bad, considering this was 80% in town (35-45mph). I installed GDE with ~6 gallons of fuel already burned, given an in-town estimate of 19-20 mpg based on prior experience (117 miles total, pre-GDE). This tank of fuel was B5, from a very sketchy place in the backwoods of Florida, which maybe wasn't the best idea

.
Also, it is important to note that I left my Jeep at my parent's house while I was fulfilling a 10-week internship assignment. The GDE tune was installed post-internship, on an old tank of sketchy biofuel

That's a recipe for some high #s right there y'all
In short, I drove an additional 340 miles on ~12 gallons of fuel post-GDE, same driving conditions. Giving me a GDE in-town average of
~28mpg, an 8mpg improvement over stock! WOOHOO!!! I can't wait to see what this puppy does on my trip next week!
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Edit 8/22
Results:
#1 - 35.3mpg, 60mph, no AC (just seeing what I could do)
#2 - 29.5mpg, 70mph, AC, lots of traffic
#3 - 29.7mpg, 70mph, AC, uphill & into a storm
#4 - 33.8mpg, 60mph, AC
Definitely an improvement over stock, although I get the feeling that GDE really shines in town more so than on the highway.